The water recovery rate reached 47% in 84 h when using the APTES-SiO2 modified membrane, while it reached only 26% in 108 h when using the virgin membrane. With a suitable design of the filtration apparatus and choice of draw solution (DS), the prepared novel TFC-FO membrane containing APTES-modified SiO2 can be used for recycling aquaculture wastewater into the DS, which can then be reused for other purposes.In many parts of the world, clean water has become increasingly scarce. Irrigation of agricultural land with treated wastewater is commonly used in response to water shortages but there is concern about the environmental fate and transport of contaminants present in the irrigation wastewater. This study aimed to examine the presence of wastewater sourced contaminants in soil and field grown corn (Zea mays) crops spray irrigated with treated wastewater. Soil, corn grain, leaves, and roots were sampled and tested from a long-term wastewater irrigation site as well as a non-irrigated control site in close geographic proximity. Samples were analyzed using comprehensive two-dimensional gas chromatography coupled to time of flight mass spectrometry (GC × GC-TOFMS) and both targeted and non-targeted analyses were conducted to determine chemical differences between the wastewater irrigated and control samples. Target compounds detected and quantified in the samples include herbicides, phthalates, and polycyclic aromatic hydrocarbons. Non-targeted analysis showed chemical differences between each the wastewater irrigated and control samples. Furthermore, new chloro-dimethyl-benzotriazole compounds, which are suspected to be transformation products created by the chlorine disinfection process of the wastewater treatment plant, were tentatively identified in the wastewater effluent. Twenty of these new benzotriazoles were detected and semi-quantified in the wastewater irrigated soil samples at a maximum concentration of 472 ng/g. Eight of the most abundant benzotriazoles were also detected in the corn roots at concentrations up to 56 ng/g.A volatile organic compound (VOC) emissions inventory of the petroleum refinery in Hebei was established. This refinery emits 1859.2 tons of VOCs per year, with wastewater collection and treatment system being the largest emissions source, accounting for 59.6% individually, followed by the recirculating cooling water system (13.4%), storage tanks (11.1%), and equipment leaks (9.4%). Organized and fugitive samples were collected simultaneously for different processes of each emissions source. A total of 100 VOC species were characterized and quantified using a gas chromatography-mass spectrometry/flame ionization detection system. The VOC emissions concentrations and chemical composition of each process were quite different. Most of the processes used alkanes as the main chemome. We concluded from the composite source profile weighted by the amount of VOC emissions that the characteristic species of this petroleum refinery were ethane (15.4%), propylene (11.7%), propane (8.5%), iso-pentane (8.3%), and toluene (4.7%). The ozone (O3) formation potential (OFP) and secondary organic aerosol formation potential (SOAP) were evaluated, and the results indicated that alkenes (mainly propylene) and aromatics (mainly toluene) were the priority control compounds. This study clarifies the current status of VOC emissions in the refinery in terms of emissions intensity, emissions components, and O3 and SOA reactivity. The key emissions sources and species screened provide scientific support for reducing refined emissions from the petrochemical industry.Studies on the symbiosis of microalgae-bacteria have been accelerating as a mean for wastewater remediation. However, there were few reports about the microalgae-bacteria consortia for chemical wastewater treatment. The aim of the present study is to develop an autotrophic and heterotrophic consortium for chemical wastewater treatment and probe whether and how bacteria could benefit from the microalgae during the treatment process, using PTA wastewater as an approach. A process-dependent strategy was applied. First of all, the results showed that the sludge beads with the sludge concentration of 30 g/L were the optimal one with the COD removal rate at 84.8% but the ceiling effect occurred (COD removal rate 92%) when LEDs light belt was offered as an advanced light condition. Biochemical assay and DNA analysis indicated that the microalgae could form an internal circulation of substances within the activated sludge and drove the microbial community to success and the corresponding gene functions, like metabolism and.Nowadays the study of the potential applications of multifunctional materials for environmental remediation is one of the main goals of the materials engineering. Multifunctional porous materials, MPMs, incorporate, all in once, different and multiple functionalities that make them suitable for several uses and can satisfy many purposes at the same time. Multifunctional diatomite-based foams with a hierarchical porosity, already produced and characterized to be applied in building as well as aerospace sectors, are proposed as adsorbents for inorganic and organic pollutants removal from wastewaters. selleck chemical Then, the effect of the addition of different carbonaceous nanofillers (graphite, graphene and graphene oxide) on the water purification efficiency of the adsorbent was evaluated. Firstly, pristine MPM showed the best performance in adsorbing Indigo Carmine due to its intrinsic chemism and hierarchical porosity (at macro-, micro- and nano-level), but it is not the best with respect to the Cd2+ adsorption, if compared with the nanocomposites. Among the nanocomposite products, both graphene- and graphene oxide-MPM samples showed a significantly improved adsorption capacity towards Cd2+. This behavior is due to the synergistic effect of the finer morphology, higher available foam surface, and the highly exfoliated fillers, graphene and graphene oxide, which permit a better dispersion into the matrix.The soil protistan community makes important contributions to the ecological functions of soil. However, our knowledge of the effects of pollutants, especially plastic particles, on the soil protistan community is still very limited compared to our knowledge on other soil microbes, such as bacterial and fungi. In this study, we revealed the effects of combined and single pollution caused by arsenic (As) and microplastics/nanoplastics (MPs/NPs) on bacterial, fungal and protistan communities. Our results revealed that combined pollution through As and MPs/NPs distinctly affected the composition and structure of the soil protistan communities (P less then 0.05), but in the case of bacteria, only some families were altered, and there was no impact on fungi. Changes of soil protistan communities might be mainly due to As pollution, and MPs/NPs exposure increased this detrimental effect. Further, As + MPs exposure greatly increased the abundance of soil protistan parasites, and As + NPs exposure caused an evident decrease in the abundance of soil protistan consumers (P less then 0.selleck chemical
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